Publication Abstracts

Sebastian et al. 2022

Sebastian, M., S.K. Kompalli, V.A. Kumar, S. Jose, S.S. Babu, G. Pandithurai, S. Singh, R.K. Hooda, V.K. Soni, J.R. Pierce, V. Vakkari, E. Asmi, D.M. Westervelt, A.-P. Hyvärinen, and V.P. Kanawade, 2022: Observations of particle number size distributions and new particle formation in six Indian locations. Atmos. Chem. Phys., 22, no. 7, 4491-4508, doi:10.5194/acp-22-4491-2022.

Atmospheric new particle formation (NPF) is a crucial process driving aerosol number concentrations in the atmosphere; it can significantly impact the evolution of atmospheric aerosol and cloud processes. This study analyses at least 1 year of asynchronous particle number size distributions at six different locations in India. We also analyze the frequency of NPF and its contribution to cloud condensation nuclei (CCN) concentrations. We found that the NPF frequency has a considerable seasonal variability. At the measurement sites analyzed in this study, NPF frequently occurs in March-May (pre-monsoon, about 21% of the days) and is the least common in October-November (post-monsoon, about 7% of the days). Considering the NPF events in all locations, the particle formation rate (JSDS) varied by more than 2 orders of magnitude (0.001-0.6 cm-3/s) and the growth rate between the smallest detectable size and 25nm (GRSDa-25nmS) by about 3 orders of magnitude (0.2-17.2 nm/h). We found that JSDS was higher by nearly 1 order of magnitude during NPF events in urban areas than mountain sites. GRSDS did not show a systematic difference. Our results showed that NPF events could significantly modulate the shape of particle number size distributions and CCN concentrations in India. The contribution of a given NPF event to CCN concentrations was the highest in urban locations (4.3×103 cm-3 per event and 1.2×103 cm-3 per event for 50 nm and 100 nm, respectively) as compared to mountain-background sites (2.7×103 cm-3 per event and 1.0×103 cm-3 per event). We emphasize that the physical and chemical pathways responsible for NPF and factors that control its contribution to CCN production require in situ field observations using recent advances in aerosol and its precursor gaseous measurement techniques.

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BibTeX Citation

@article{se02300g,
  author={Sebastian, M. and Kompalli, S. K. and Kumar, V. A. and Jose, S. and Babu, S. S. and Pandithurai, G. and Singh, S. and Hooda, R. K. and Soni, V. K. and Pierce, J. R. and Vakkari, V. and Asmi, E. and Westervelt, D. M. and Hyvärinen, A.-P. and Kanawade, V. P.},
  title={Observations of particle number size distributions and new particle formation in six Indian locations},
  year={2022},
  journal={Atmos. Chem. Phys.},
  volume={22},
  number={7},
  pages={4491--4508},
  doi={10.5194/acp-22-4491-2022},
}

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RIS Citation

TY  - JOUR
ID  - se02300g
AU  - Sebastian, M.
AU  - Kompalli, S. K.
AU  - Kumar, V. A.
AU  - Jose, S.
AU  - Babu, S. S.
AU  - Pandithurai, G.
AU  - Singh, S.
AU  - Hooda, R. K.
AU  - Soni, V. K.
AU  - Pierce, J. R.
AU  - Vakkari, V.
AU  - Asmi, E.
AU  - Westervelt, D. M.
AU  - Hyvärinen, A.-P.
AU  - Kanawade, V. P.
PY  - 2022
TI  - Observations of particle number size distributions and new particle formation in six Indian locations
JA  - Atmos. Chem. Phys.
VL  - 22
IS  - 7
SP  - 4491
EP  - 4508
DO  - 10.5194/acp-22-4491-2022
ER  -

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