Publication Abstracts
Reidmiller et al. 2009
Reidmiller, D.R., A.M. Fiore, D.A. Jaffe, D. Bergmann, C. Cuvelier, F.J. Dentener, B.N. Duncan, G. Folberth, M. Gauss, S. Gong, P. Hess, J.E. Jonson, T. Keating, A. Lupu, E. Marmer, R. Park, M.G. Schultz, , S. Szopa, M.G. Vivanco, O. Wild, and A. Zuber, 2009: The influence of foreign vs. North American emissions on surface ozone in the US. Atmos. Chem. Phys., 9, 5027-5042, doi:10.5194/acp-9-5027-2009.
As part of the Hemispheric Transport of Air Pollution (HTAP; http://www.htap.org/) project, we analyze results from 16 global and hemispheric chemical transport models and compare these to Clean Air Status and Trends Network (CASTNet) observations in the United States (US) for 2001. Using the policy-relevant maximum daily 8-h ozone (MDA8 O3) statistic, the multi-model ensemble represents the observations well (mean r2=0.57, ensemble bias=+4.1 ppbv for all regions and all seasons) despite a wide range in the individual model results. Correlations are strongest in the NorthEastern US during spring and fall (r2=0.68); and weakest in the Midwestern US in summer (r2=0.46). However, large positive mean biases exist during summer for all Eastern US regions, ranging from 10-20 ppbv, and a smaller negative bias is present in the Western US during spring (∼3 ppbv). In most all other regions and seasons, the biases of the model ensemble simulations are ≤ 5 ppbv. Sensitivity simulations in which anthropogenic O3-precursor emissions (NOx+NMVOC+CO+aerosols) were decreased by 20% in each of four source regions: East Asia (EA), South Asia (SA), Europe (EU) and North America (NA) show that the greatest response of MDA8 O3 to the summed foreign emissions reductions occurs during spring in the West (0.9 ppbv reduction due to 20% reductions from EA+SA+EU). East Asia is the largest contributor to MDA8 O3 at all ranges of the O3 distribution for most regions (typically ∼0.45 ppbv). The exception is in the NorthEastern US where European emissions reductions had the greatest impact on MDA8 O3, particularly in the middle of the MDA8 O3 distribution (response of ∼0.35 ppbv between 35-55 ppbv). In all regions and seasons, however, O3-precursor emissions reductions of 20% in the NA source region decrease MDA8 O3 the most — by a factor of 2 to nearly 10 relative to foreign emissions reductions. The O3 response to anthropogenic NA emissions is greatest in the Eastern US during summer at the high end of the O3 distribution (5-6 ppbv for 20% reductions). While the impact of foreign emissions on surface O3 in the US is not negligible — and is of increasing concern given the growth in emissions upwind of the US — domestic emissions reductions remain a far more effective means of decreasing MDA8 O3 values, particularly those above 75 ppb (the current US standard).
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BibTeX Citation
@article{re05000n,
author={Reidmiller, D. R. and Fiore, A. M. and Jaffe, D. A. and Bergmann, D. and Cuvelier, C. and Dentener, F. J. and Duncan, B. N. and Folberth, G. and Gauss, M. and Gong, S. and Hess, P. and Jonson, J. E. and Keating, T. and Lupu, A. and Marmer, E. and Park, R. and Schultz, M. G. and Shindell, D. T. and Szopa, S. and Vivanco, M. G. and Wild, O. and Zuber, A.},
title={The influence of foreign vs. North American emissions on surface ozone in the US},
year={2009},
journal={Atmospheric Chemistry and Physics},
volume={9},
pages={5027--5042},
doi={10.5194/acp-9-5027-2009},
}
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RIS Citation
TY - JOUR ID - re05000n AU - Reidmiller, D. R. AU - Fiore, A. M. AU - Jaffe, D. A. AU - Bergmann, D. AU - Cuvelier, C. AU - Dentener, F. J. AU - Duncan, B. N. AU - Folberth, G. AU - Gauss, M. AU - Gong, S. AU - Hess, P. AU - Jonson, J. E. AU - Keating, T. AU - Lupu, A. AU - Marmer, E. AU - Park, R. AU - Schultz, M. G. AU - Shindell, D. T. AU - Szopa, S. AU - Vivanco, M. G. AU - Wild, O. AU - Zuber, A. PY - 2009 TI - The influence of foreign vs. North American emissions on surface ozone in the US JA - Atmos. Chem. Phys. JO - Atmospheric Chemistry and Physics VL - 9 SP - 5027 EP - 5042 DO - 10.5194/acp-9-5027-2009 ER -
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