Publication Abstracts

Orbe et al. 2021, accepted

Orbe, C., D.W. Waugh, S. Montzka, E.J. Dlugokencky, S.E. Strahan, S.D. Steenrod, S. Strode, J.W. Elkins, B. Hall, C. Sweeney, E.J. Hinsta, F.L. Moore, and E. Penafiel, 2021: Tropospheric age-of-air: Influence of SF6 emissions on recent surface trends and model biases. J. Geophys. Res. Atmos., accepted.

The mean age since air was last at the Northern Hemisphere (NH) midlatitude surface is a fundamental property of tropospheric transport. Here we approximate the mean age in terms of an "SF6 age" (ΓSF6), derived from surface and aircraft measurements of SF6 that are broader in spatial scope and cover a longer time period (1997-2018) than considered previously. At the surface, ΓSF6 increases from near-zero values north of 30°N to ∼1.5 years over the Southern Hemisphere (SH) extratropics, with the largest meridional gradients occurring in the tropics. By comparison, vertical gradients in ΓSF6 are weak throughout, with only slight increases/decreases with height in the NH/SH. The broader spatial coverage of the measurements reveals strong variations in the seasonal cycle of ΓSF6 within the (sub)tropics that are weaker over the Atlantic and Pacific oceans, compared to over the Indian Ocean.

Observations from 2000-2018 reveal that the SF6 age at sites in the SH has been decreasing by ∼0.12 yr/dec. However, this decrease is not due to changes in transport but, rather, is likely related to changes in emissions, which have increased globally and reportedly shifted from northern midlatitudes into the subtropics. Simulations, which reproduce the SF6 age trends, show no decreases in an age-of-air tracer, reinforcing the fact that ΓSF6 represents only an approximation to the mean age. Finally, the modeled SF6 ages are older than observed, by ∼0.3-0.4 years throughout the southern extratropics. We show that this bias is partly related to an overestimation in simulated SF6 near emissions regions.

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BibTeX Citation

@unpublished{or03200x,
  author={Orbe, C. and Waugh, D. W. and Montzka, S. and Dlugokencky, E. J. and Strahan, S. E. and Steenrod, S. D. and Strode, S. and Elkins, J. W. and Hall, B. and Sweeney, C. and Hinsta, E. J. and Moore, F. L. and Penafiel, E.},
  title={Tropospheric age-of-air: Influence of SF6 emissions on recent surface trends and model biases},
  year={2021},
  journal={J. Geophys. Res. Atmos.},
}

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RIS Citation

TY  - INPR
ID  - or03200x
AU  - Orbe, C.
AU  - Waugh, D. W.
AU  - Montzka, S.
AU  - Dlugokencky, E. J.
AU  - Strahan, S. E.
AU  - Steenrod, S. D.
AU  - Strode, S.
AU  - Elkins, J. W.
AU  - Hall, B.
AU  - Sweeney, C.
AU  - Hinsta, E. J.
AU  - Moore, F. L.
AU  - Penafiel, E.
PY  - 2021
TI  - Tropospheric age-of-air: Influence of SF6 emissions on recent surface trends and model biases
JA  - J. Geophys. Res. Atmos.
ER  -

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