Publication Abstracts
Mishchenko et al. 2013
, , and D.W. Mackowski, 2013: T-matrix modeling of linear depolarization by morphologically complex soot and soot-containing aerosols. J. Quant. Spectrosc. Radiat. Transfer, 123, 135-144, doi:10.1016/j.jqsrt.2012.11.012.
We use state-of-the-art public-domain Fortran codes based on the T-matrix method to calculate orientation and ensemble averaged scattering matrix elements for a variety of morphologically complex black carbon (BC) and BC-containing aerosol particles, with a special emphasis on the linear depolarization ratio (LDR). We explain theoretically the quasi-Rayleigh LDR peak at side-scattering angles typical of low-density soot fractals and conclude that the measurement of this feature enables one to evaluate the compactness state of BC clusters and trace the evolution of low-density fluffy fractals into densely packed aggregates. We show that small backscattering LDRs measured with ground-based, airborne, and spaceborne lidars for fresh smoke generally agree with the values predicted theoretically for fluffy BC fractals and densely packed near-spheroidal BC aggregates. To reproduce higher lidar LDRs observed for aged smoke, one needs alternative particle models such as shape mixtures of BC spheroids or cylinders.
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BibTeX Citation
@article{mi09810t, author={Mishchenko, M. I. and Liu, L. and Mackowski, D. W.}, title={T-matrix modeling of linear depolarization by morphologically complex soot and soot-containing aerosols}, year={2013}, journal={J. Quant. Spectrosc. Radiat. Transfer}, volume={123}, pages={135--144}, doi={10.1016/j.jqsrt.2012.11.012}, }
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RIS Citation
TY - JOUR ID - mi09810t AU - Mishchenko, M. I. AU - Liu, L. AU - Mackowski, D. W. PY - 2013 TI - T-matrix modeling of linear depolarization by morphologically complex soot and soot-containing aerosols JA - J. Quant. Spectrosc. Radiat. Transfer VL - 123 SP - 135 EP - 144 DO - 10.1016/j.jqsrt.2012.11.012 ER -
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